Photofission
measurements enable selective
investigation of the extremely deformed nuclear states in the light
actinides and can be utilized to better understand the landscape of
the multiple-humped potential energy surface in these nuclei.
The selectivity of these measurements originates from the low and
reasonably well-defined amount of angular momentum transferred during
the photoabsorption process. So far, fission resonances have
been studied primarily in light-particle-induced nuclear reactions. These studies do not benefit from the same selectivity
found in photonuclear excitation and consequently they are
complicated by statistical population of the states in the 2nd
and 3rd
minima with a very limited probability of. These measurements have also suffered from
dominating prompt-fission background.
Until
now, sub-barrier photofission experiments have been performed only
with bremsstrahlung photons and have determined only the integrated
fission yield. In these experiments, the fission cross section is
convolved with the spectral intensity of the photon beam, resulting
in a typical effective γ-ray
bandwidth ΔE/E
between only 300-400 keV.
These experiments observe a plateau, referred to as the "isomeric
shelf",
in the fission cross section, presumably as a result of the
competition between prompt and delayed photofission. However,
due to the lack of high resolution photofission studies in the
corresponding energy region (E≈4-5 MeV), no experimental
information exists to confirm this concept.
Higher-resolution
studies could be performed at tagged-photon facilities (e.g. NEPTUN
at Darmstadt, Germany), though only with marginal statistics, due to
the limited beam intensities realizable through tagging, ~104
γ/(keVs)
[13]. This beam intensity cannot be significantly improved, since it
is determined by the random coincidence contribution in the
electron-tagging process. Thus, high statistics photofission
experiments in the deep sub-barrier energy region, where cross
sections are typically as low as σ=1
nb-10 μb,
cannot be performed with tagged-photon beams.
The
relatively recent development of inverse-Compton scattering γ-ray
sources, capable of producing tunable, high-flux, quasi-monoenergetic
γ-ray
beams by Compton-backscattering of eV-range photons off a
relativistic electron beam, offers an opportunity to overcome
previous limitations. It has to be emphasized that a measurement of
the photofission cross section in the deep sub-barrier energy region
will be a crucial step towards a reliable characterization of the
PES, including unambiguous determination of the double- or
triple-humped nature of the surface and precise evaluation of the
barrier parameters.
Currently,
the most intense Compton-backscattered γ-ray
source is the High Intensity γ-ray
Source (HIγS)
at the Duke University (USA) with a bandwidth
of
ΔE=150-200
keV and a spectral flux of 102
γ/(eVs).
Next-generation
Compton-backscattering γ-ray
sources, such as the upgrade of HIγS
(HIγS2),
and
the Extreme LIght Infrastructure - Nuclear Physics (ELI-NP, Bucharest, Romania), are anticipated to provide beams
with spectral fluxes up to ~106
γ/(eVs)
and energy resolutions down to ΔE~1
keV, far superior to those currently available at presently available
γ
sources. The capabilities of these next-generation sources allow one
to aim at an identification of low-amplitude fission resonances. The narrow energy bandwidth expected for the new
γ
beam facilities will also allow for a significant reduction of the
presently dominant background from non-resonant processes. Thus, next-generation γ-ray
sources are expected to enable observation of the fine structure in
the isomeric shelf. This
may open the perspective towards a new era of photofission studies.